Thermalization dynamics in a pulsed microwave plasma-enhanced laminar flame
نویسندگان
چکیده
Energy transfer in a pulsed-microwave enhanced flame is investigated using hybrid fs/ps coherent anti-Stokes Raman scattering (CARS) to monitor both vibrational and rotational temperatures of nitrogen an atmospheric pressure laminar premixed natural gas/air stagnation flame. Temperatures were measured throughout the structure following 30-kW peak power, 2 ?s duration, 3 GHz microwave pulse resonant waveguide cavity. CARS measurements show delayed increase temperature, indicating energy loading via electron impact subsequent cascade. Vibrational thermalization was observed over timescales faster than transport through zone, but slower predicted by known vibrational-translational rates, suggesting long-lived pathway for increased temperature. Peak temperature increases 100 K thermalize 100?s microseconds, resulting measurable same time interval. The magnitude excitation rate such plasma-assisted combustion environments critical applications including ignition control, provide necessary detail on relaxation processes ground state nitrogen.
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ژورنال
عنوان ژورنال: Combustion and Flame
سال: 2021
ISSN: ['1556-2921', '0010-2180']
DOI: https://doi.org/10.1016/j.combustflame.2021.01.006